This download looks like an addon. You need to extract the downloaded zip and put the addon folder in your Garry's Mod addons folder. You should end up with a directory structure similar to below:
Don't know where the Garry's Mod folder is or how to extract zip files? See more useful installation tips.
mossesx, Sparkle Spy Box Trot (Orange), Xlion315, sandman, jamIn, The Scurvy Orange, bind "mouse1" "kill", Mexari, in space noone can hear you fart, Casey, Deviant Pengu, SchwarzeTrauer, Frost1551, DecoyofChivalry, beta50test, DR.WCROW, DR.WCROW, Ghost Pancakes, Ichiro Higashiyama, Ichiro Higashiyama, PeculiarReality