This download looks like an addon. You need to extract the downloaded zip and put the addon folder in your Garry's Mod addons folder. You should end up with a directory structure similar to below:
Don't know where the Garry's Mod folder is or how to extract zip files? See more useful installation tips.
Sashaukrainian9, 1829724793, 1829724793, Mleonel2009, pedroelisioteixeira, 2162216617, rohanking1685, Erikdudi127, Pyro_gaming, johnsonkamir7, machinesplays_gquis, Hyperloquendo1, 886, kbaranyigitkizgin, AndrestheMiner, Aige, gordon freeman, Tortall, winterjr552, monir, DeltaGreninja77TF2EASY.COM, spacecatalpha, Omphy, v4ceslav12, dhauhedhniah, bbr29, fisak345fangrop, fisak345fangrop, ossaj2.day72, 福建舰 福建见, Usiqyk, Mr. Heck, wasa399, Juzek z Bagien, MrARTOS, artemskv49gmail.com, tema-dnk, неизвестен, неизвестен, неизвестен, MenaceKPlayz, naru38games, cnc_2014, Dark↙↙[A]tk, nohitounmei, telewizor100 KeyDrop.com, scp84239, shuminanazarova-2011, Allan, FlyingKitty +353 others